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最新综述:碳基非金属催化剂具有许多优点,如高地球丰度、低成本、高导电性、结构可调、选择性好、在酸性或碱性条件下稳定性强以及绿色环保等。由于这些特性,这些催化剂最近在能源和环境领域的应用中受到越来越多的关注。随后,各种碳基催化剂已发展到可替代贵金属催化剂,用于低成本可再生清洁与环保能源的生产与存储。针对这个快速发展的领域,本文综述了其最新重要研究进展,包括机理认识、结构设计、用于清洁能源转换与存储且环保的碳基非金属电催化剂材料/器件的制备以及对目前挑战与前景的讨论。
Abstract: Carbon-based metal-free catalysts possess desirable properties such as high earth abundance, low cost, high electrical conductivity, structural tunability, good selectivity, strong stability in acidic/alkaline conditions, and environmental friendliness. Because of these properties, these catalysts have recently received increasing attention in energy and environmental applications. Subsequently, various carbon-based electrocatalysts have been developed to replace noble metal catalysts for low-cost renewable generation and storage of clean energy and environmental protection through metal-free electrocatalysis. This article provides an up-to-date review of this rapidly developing field by critically assessing recent advances in the mechanistic understanding, structure design, and material/device fabrication of metal-free carbon-based electrocatalysts for clean energy conversion/storage and environmental protection, along with discussions on current challenges and perspectives.
文章介绍
The review is included in the issue 1, vol.1, 2018 of EER. Please refer to the following link from more detailed information, and the full text is freely downloadable.
Article Title:Carbon-Based Metal-Free Electrocatalysis for Energy Conversion, Energy Storage, and Environmental Protection
Cite as:Hu, C., Xiao, Y., Zou, Y. et al. Electrochem. Energ. Rev. (2018) 1: 84. https://doi.org/10.1007/s41918-018-0003-2
Keywords: Metal-free electrocatalysis · Carbon-based catalysts · Energy conversion and storage · Environmental protection
Full text:https://link.springer.com/article/10.1007/s41918-018-0003-2/fulltext.html
原文(扫描或长按二维码,识别后直达原文页面):
Biographies of Authors
Chuangang Hu (first author) received his MS from Henan Normal University in 2011, and his Ph.D. from Beijing Institute of Technology in 2015. He is currently a postdoctoral research associate in Professor Liming Dai’s group at Case Western Reserve University. His research interests focus on carbon-based materials for energy conversion and storage.
Ying Xiao received her PhD degree from Beijing Insinuate of Technology in 2015. From December of 2015 to December of 2016, she was a postdoctoral researcher at Hanyang University. She is currently a postdoctoral researcher at BUCT-CWRU International Joint Lab. Her current research interests focus on the design and synthesis of carbon- based materials and their applications in metal-air batteries.
Yuqin Zou received her bachelor and master’s degree in 2012 from Shanghai University and her Ph.D. in 2017 from The University of Manchester. She is currently a lecturer of the College of Energy, Beijing University of Chemical Technology. Her research interests are in novel 2D materials, such as graphene, layered double hydroxide and black phosphorus, and their application in energy storages devices and electrocatalysis.
Liming Dai (corresponding author) joined Case Western Reserve University (CWRU) in fall 2009 as the Kent Hale Smith Professor in the Department of Macromolecular Science and Engineering. He is also director of the Center of Advanced Science and Engineering for Carbon (CASE4Carbon). Dr. Dai received a B.Sc. degree from Zhejiang University in 1983, and a Ph.D. from the Australian National University in 1991. He accepted a postdoctoral fellowship from the Cavendish Laboratory at the University of Cambridge and two years later became a visiting follow at the University of Illinois at Urbana-Champaign. Dr. Dai’s expertise lies across the synthesis, chemical modification and device fabrication of conjugated polymers and carbon nanomaterials for energy-related and biomedical applications.
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Electrochemical Energy Reviews (《电化学能源评论》,简称EER),该期刊旨在及时反映国际电化学能源转换与存储领域的最新科研成果和动态,促进国内、国际的学术交流,设有专题综述和一般综述栏目。EER是国际上第一本专注电化学能源的综述性期刊。EER覆盖化学能源转换与存储所有学科,包括燃料电池,锂电池,金属-空气电池,超级电容器,制氢-储氢,CO2转换等。
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